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81.
Extensive organic-matter (OM) rich facies (black shales) occur in the Ordo-Silurian boundary successions in the Yangtze area, South China. To investigate the redox changes of the Yangtze Sea during the Ordo-Silurian transition, two OM sections (Wangjiawan in Yichang, Hubei Province, and Sanjiaguan in Zhangjiajie, Hunan Province) straddling the Ordo-Silurian boundary are studied. The measurements finished in this study include contents of the total organic carbon (TOC), pyrite sulphur, and different species of Fe, including dithionite-extractable Fe (FED), pyrite Fe (FeP), HCl-extractable Fe (FeH), and total Fe (FeT), in black shales, as well as other redox proxies, such as the SIC ratio, the ratio between highly reactive Fe (FeHR = FeD + FeP) and FeT, and the FeP/(FeP + FeH) ratio, known as the degree of pyritization (DOP). In the Wangjiawan section, the Middle Ashgill sediments have high FeHR/FeT ratios (0.20-0.77; avg. 0.45), high DOP values (0.21-0.72; avg. 0.54), and a relatively constant sulfur content independent of the organic carbon content. By the contrast, the mid-early Hirnantian deposits generally have low FeHR/FeT ratios (0.10-0.35; avg. 0.21), low DOP values (0.11- 0.40; avg. 0.28), and SIC values are clustering on the normal marine value (SIC = 0.36). The late Hirnantian and early Rhuddanian deposits, similar to those of the Middle Ashgill deposits, are characterized by high FeHR/FeT ratios (0.32-0.49; avg. 0.41), high DOP values (0.46-0.68; avg. 0.53) and fairly constant sulfur contents. These data suggest the occurrences of marine anoxia on the Yangtze Sea shelf during intervals of the Mid Ashgill, Late Hirnantian and Early Rhuddanian, and ventilated and oxygenated marine conditions during the mid-early Hirnantian time. The mid-early Hirnantian ventilated event was concomitant with the global glacial period, likely resulted from the glacio-eustatic sea-level fall and subsequent circulation of cold, dense oxygenated waters 相似文献
82.
北京市土壤Hg污染的区域生态地球化学评价 总被引:8,自引:1,他引:7
城市土壤Hg异常/污染是中国普遍存在的重大生态环境问题。文章对北京市近1000km2范围内的地表土壤、壤中气、大气干湿沉降、大气颗粒物、大气中的Hg含量水平和空间分布模式进行了系统研究,查明北京地表土壤Hg平均含量为0.41mg/kg,大气干湿沉降物中的Hg平均含量为0.194mg/kg,壤中气Hg的平均含量为559.65ng/m3,大气颗粒物PM10和PM2.5中的Hg含量分别为0.59和0.67ng/m3,大气中的Hg平均含量为3.13ng/m3。北京市自2000年起实现了由燃煤转变为燃气的减排措施,导致干湿沉降物中的Hg沉降通量显著减少,2006年大气干湿沉降物中Hg的沉降通量1.837mg·m-2·a-1,北京市城区(近1000km2)Hg全年沉降为1837kg,空气中总Hg浓度由1998年的8.3~24.7ng/m3下降到2006年的3.13ng/m3,大气颗粒物中Hg含量由2003年的1.18ng/m3下降到2006年的0.59ng/m3(PM10)和0.67ng/m3(PM2.5),表明北京市煤改气减排措施的实施显著改善了大气环境质量。通过对土壤中Hg的存在形式研究,发现土壤中有硫化物(辰砂)及各种Hg盐(HgCl2)的含Hg矿物,Hg也可以各种吸附方式或壤中气方式存在。研究证实北京壤中气Hg与大气Hg存在显著的相关性(n=131,R=0.267,p<0.01),表明壤中气Hg是大气Hg的重要来源之一。利用2005年地表土壤总Hg与Hg释放速率的线性方程估算,土壤Hg平均释放速率为102.42ng·m-2·h-1,2005年土壤释放进大气的Hg通量为936.70kg。在查明土壤中存在大量辰砂矿物的同时,还分布有大量具有高温熔融特征的金属微球粒和玻璃质微球粒,证明燃煤和冶金烟尘是地表土壤Hg的主要来源。土壤中Hg、S、pH和辰砂颗粒浓度在空间上的高度耦合性表明,碱性条件下,土壤中高含量的S和Hg是辰砂形成的重要原因。按国家土壤环境质量标准,北京市I级土壤Hg环境质量的面积为176km2,Ⅱ级为808km2,Ⅲ级为24km2,超Ⅲ为36km2。Ⅲ级、超Ⅲ级主要分布在二环路以内的中心城区。城南(长安街为界)大气Hg环境质量明显优于城北,在北四、北五环之间的部分地区,大气颗粒Hg的环境质量为Ⅲ级或超Ⅲ级。在地表土壤Hg含量较高的中心城区,居民每天因呼吸摄入的Hg高达364ng,对人体健康构成潜在风险。根据我国"十一五"规划中每年实现10%节能减排的目标,对北京市未来50年土壤Hg含量的时空演变趋势预测,预测2050年北京因干湿沉降带来的Hg输入量为16.03kg,地表土壤释放Hg的输出量为37.36kg,明显大于Hg的输入通量,土壤Hg的环境质量将得到根本改善。预测到2040年Ⅲ级土壤Hg环境质量的区域将完全消失,到2060年以Ⅰ级土壤为主。 相似文献
83.
Sukanta Roy Labani Ray Anurup Bhattacharya R. Srinivasan 《International Journal of Earth Sciences》2008,97(2):245-256
The Late Archaean Closepet Granite batholith in south India is exposed at different crustal levels grading from greenschist
facies in the north through amphibolite and granulite facies in the south along a ∼400 km long segment in the Dharwar craton.
Two areas, Pavagada and Magadi, located in the Main Mass of the batholith, best represent the granitoid of the greenschist
and amphibolite facies crustal levels respectively. Heat flow estimates of 38 mW m−2 from Pavagada and 25 mW m−2 from Magadi have been obtained through measurements in deep (430 and 445 m) and carefully sited boreholes. Measurements made
in four boreholes of opportunity in Pavagada area yield a mean heat flow of 39 ± 4 (s.d.) mW m−2, which is in good agreement with the estimate from deep borehole. The study, therefore, demonstrates a clear-cut heat flow
variation concomitant with the crustal levels exposed in the two areas. The mean heat production estimates for the greenschist
facies and amphibolite facies layers constituting the Main Mass of the batholith are 2.9 and 1.8 μW m−3, respectively. The enhanced heat flow in the Pavagada area is consistent with the occurrence of a radioelement-enriched 2-km-thick
greenschist facies layer granitoid overlying the granitoid of the amphibolite facies layer which is twice as thick as represented
in the Magadi area. The crustal heat production models indicate similar mantle heat flow estimates in the range 12–14 mW m−2, consistent with the other parts of the greenstone-granite-gneiss terrain of the Dharwar craton. 相似文献
84.
85.
86.
Carsten Blindauer Vladimir Rozanov John Philip Burrows 《Journal of Atmospheric Chemistry》1996,24(1):1-21
The accurate radiative transfer model GOMETRAN, initially designed to yield radiances at TOA in the wavelength range 240–790 nm, has been extended to allow for the computation of actinic fluxes down to 175 nm and for the calculation of photolysis frequencies in the atmosphere. The capability of the extended model PHOTOGT (PHOTOGOMETRAN) is demonstrated in a number of successful comparison studies both with recent experiments (ground-based, balloonborne, airborne) and model calculations of radiances, actinic fluxes and photolysis frequencies in the stratosphere and troposphere. In an atmospheric case study, the impact of new quantum yield data for the O3 » O2+O(1
d) photodissociation channel on the photolytic production of O(1
d) atoms in the lower atmosphere has been quantified. 相似文献
87.
Jacek A. Majorowicz 《Pure and Applied Geophysics》1996,147(1):1-24
The results of precision temperature logs made to depths of several hundred meters in some 80 wells in Western Canada, most of which are located in the Prairie Provinces, show evidence of warming at the ground surface in the 0.5 K to 3.5 K range (average=2.2±0.7 K, for 80 unevenly distributed sites). Modeling shows that this warming mostly pertains to this century and it has been most substantal in the last four decades if the ramp function of the linear increase of surface temperature is assumed. Using the step function model's increase of surface temperature (land clearing, forest fires, etc.) the calculated onset of warming would pertain mostly to the last two decades. Contour maps of ground temperatures currently and previously and a contour map of the ground warming magnitude dilineate a large regional character of the ground temperature change at the southern marigin of permafrost for the large area of the Prairie Provinces. In many cases however, the magnitude of ground warming is much larger than the magnitude of air warming. This is especially evident for the northern areas of Alberta in the boreal forest ecoprovince. The magnitude of ground warming is equal to the magnitude of surface air warming in southern Alberta in the grassland and aspen parkland ecoprovinces. The analysis of the temperature depth response to the surface warming from well data shows the integrated effect of surface air warming together with the increases in ground temperature due to natural terrain effects and other anthropogenical changes to the surface of the earth. 相似文献
88.
High frequency temperature measurements were recorded at five heights and surface renewal (SR) analysis was used to estimate sensible heat flux density (H) over 0.1 m tall grass. Traces of the temperature data showed ramp-like structures, and the mean amplitude and duration of these ramps were used to calculate H using structure functions. Data were compared with H values measured with a sonic anemometer. Latent heat flux density (E) was calculated using an energy balance and the results were compared with E computed from the sonic anemometer data. SR analysis provided good estimates of H for data recorded at all heights but the canopy top and at the highest measurement level, which was above the fully adjusted boundary layer. 相似文献
89.
A dynamic box model was applied to study the characteristics of biogeochemical cycling of PO_4-P,NO_3-N,AOU,POC and PON in the southern Taiwan Strait region based on field data of the"Minnan Taiwan Bank Fishing Ground Upwelling Ecosystem Study" during the period of Dec.1987-Nov.1988.According to the unique hydrological and topographical features of the region,six boxesand three layers were considered in the model.The variation rates and fluxes of elements induced by hor-izontal current,upwelling,by diffusion,sinking of particles and biogeochemical processes were estimatedrespectively.Results further confirmed that upwellings had important effects in this region.Thenearshore upwelling areas had net input fluxes of nutrients brought by upwelling water,also had high de-pletion rates of nutrients and production rates of particulate organic matter and dissolved oxygen.Theabnormal net production of nutrients in the middle layer(10-30m) indicated the important role of bacte-ria in this high production region.Th 相似文献
90.
钻遇莫霍面是人类一直以来的梦想。深海海底是地球上离莫霍面最近的地方,目前有研究推测南海是世界上莫霍面深度最浅的海域之一,但缺乏足够的直接证据。深反射地震探测可以直接揭示岩石圈的构造形态,是莫霍面探测的重要手段。本文基于长达15000 km的深反射多道地震剖面的解释、处理、制图和分析,结合前人的研究,形成了南海海盆区莫霍面反射特征和空间分布的初步认识。① 南海东部次海盆南部早期经历了较快速扩张,岩浆供应充足,受扩张停止后岩浆活动影响较小,基底平坦,地质构造相对简单,同时洋壳地震速度结构不存在异常,且有较强的广角莫霍面反射波和可识别的地幔顶部折射波,具备莫霍面钻探的基本条件。② 南海海盆不同区域的莫霍面反射强度存在较大差异。其中东部次海盆莫霍面反射最为强烈且清晰,西北次海盆次之,西南次海盆仅有零星出现的清晰莫霍面反射且可信度不高。③ 识别南海海盆区莫霍面地震反射长度超过3500 km,首次形成了海盆区深度域莫霍面地震反射空间分布图。与重力反演的莫霍面深度相比,利用深反射多道地震计算的莫霍面深度细节更为丰富,并且可以在垂向上清晰刻画莫霍面的结构。整体上,南海海盆区莫霍面地震反射强烈和可信度高的区域中,深度较浅的区域之一是东部次海盆南部,最浅处仅约9. 5 km,其中水深4. 01 km,洋壳厚度仅5. 54 km。综合判断,东部次海盆南部是南海重要的莫霍面钻探备选区,这对南海莫霍面钻探选址具有重要意义。 相似文献